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The THz pump is generated by optical rectification in the DSTMS crystal, whereas the probe light is splitted from the infrared that drives the THz pulse. The two copropagating beams are synchronized by a delay line stage and are incident onto the 2-μm-thick, 100-cut silicon crystal at a normal angle. Even-order harmonics generation from the Si crystal is detected in transmission by a spectrometer. The x, y, and z axes are defined in the laboratory frame, where the y axis is parallel to the (100). In order to avoid unnecessary infrared energy leaked from the DSTMS crystal, a Teflon plate is placed behind the DSTMS to block the infrared light. 153554b96e
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